Read e-book online Alternative Fuels Guidebook PDF

By Bechtold R.L.

ISBN-10: 0768000521

ISBN-13: 9780768000528

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The x axis parallel to the surface plane using the notation of Fig. 4. This explanation differs from the original one proposed by Kazusaka et u1. (61), who appear not to have made the correct choice for the axis system. ]: N MOLECULAR OXYGEN SPECIES ON OXIDE SURFACES 27 Vedrine et al. 01 12, and A , = 24, A , = 66, A , = 12 G . However, inspection of the published spectra indicates that A , and A , are difficult to estimate. , they axis in Fig. 4. This is difficult to reconcile with the observed orthorhombic g and A tensors, which are not averaged.

Two explanations for this observation are possible (Fig. 8). One is that these splittings refer to oxygen nuclei in two 0; ions in different surface sites (case 1); the other is that they refer to two oxygen nuclei in the same 0;(case 2) (82, 85). In general, if two different types of 0; are present, they should lead to two sets of g tensors. 21 I Case 2 Equivalent sites. different nuclei I I 0; with both nuclei labeled I I FIG 8 Configuration for inequivalent oxygen nuclei in the 0, ion (85) distinguished.

In this situation, the outermost oxygen (B in Fig. 8) is assumed to have the largest spin density by analogy with the results from linewidth studies (94h) and selective isotopic labeling (95) for the organic peroxy radicals. The reasons for this kind of adsorption are not clear and they probably depend on two main factors: the topology of the surface and/or the nature of the orbital at the adsorption site available to overlap with the n: orbitals of oxygen. The first factor has been favored by Che et al.

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Alternative Fuels Guidebook by Bechtold R.L.

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